A silicon mould will accept pretty much any material or texture you want, as Dewbakuk has already stated.
Silicon is a wonderful material to work with, and once you learn how to use it and your resin mix, you can make lots of copies of your work.
For the mould walls, lego blocks seem to be a popular choice (never tryed them myself), or you can make them with plasticard, but for your first attempts, simple and cheap child's modelling clay will work too.
Hope that helps.